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Experimental evidence of a dynamic Jahn-Teller effect in C-60 (+)
Abstract
Detailed analysis of the HOMO bandshape in the photoelectron spectrum of gaseous C60 reveals a dynamic Jahn-Teller effect in the ground state of C60+. The direct observation of three tunneling states asserts a D3d geometry for the isolated cation, originating from a strong vibronic coupling. These results show that the ionic motion of the ions plays an important role in the electron-phonon interaction.
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