UC Irvine

Superconducting qubits are hampered by flux noise produced by surface spins from a variety of microscopic sources. Recent experiments indicated that hydrogen (H) atoms may be one of those sources. Using density functional theory calculations, we report that H atoms either embedded in, or adsorbed on, an α-Al2O3(0001) surface have sizable spin moments ranging from 0.81 to 0.87μB with energy barriers for spin reorientation as low as ∼10mK. Furthermore, H adatoms on the surface attract gas molecules such as O2, producing new spin sources. We propose coating the surface with graphene to eliminate H-induced surface spins and to protect the surface from other adsorbates.