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Thermally induced metal-to-insulator transition in NbO2 thin films: Modulation of the transition temperature by epitaxial strain

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https://journals.aps.org/prmaterials/abstract/10.1103/PhysRevMaterials.3.124602
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Abstract

Modification of the carrier dynamics in correlated oxide systems via epitaxial strain is a promising pathway for the practical realization of energy-efficient electronic devices. Here we report on the thermally induced metal-to-insulator transition (MIT) of NbO2 films grown on Al2O3 substrates and the modulation of the MIT temperature via epitaxial strain from the substrate. The metal-insulator transition temperature (TMIT) increased from 910 to 1066 K with increasing strain. An ultrathin 3.9-nm film consisting of a single strained layer with minimal structural defects yielded a bulklike sharp transition. The substrate-induced strain offers another degree of freedom to improve device functionality of MIT materials.

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