- Ziemkiewicz, David;
- Knez, David;
- Garcia, Evan P;
- Zielińska-Raczyńska, Sylwia;
- Czajkowski, Gerard;
- Salandrino, Alessandro;
- Kharintsev, Sergey S;
- Noskov, Aleksei I;
- Potma, Eric O;
- Fishman, Dmitry A
Two-photon absorption in indirect gap semiconductors is a frequently encountered, but not well-understood phenomenon. To address this, the real-density matrix approach is applied to describe two-photon absorption in silicon through the excitonic response to the interacting fields. This approach produces an analytical expression for the dispersion of the two-photon absorption coefficient for indirect-gap materials and can be used to explain trends in reported experimental data for bulk silicon both old and new with minimal fitting.