In recent models, the neutron-rich Ni isotopes around N=40 are predicted to exhibit multiple low-energy excited 0+ states attributed to neutron and proton excitations across both the N=40 and Z=28 shell gaps. In Ni68, the three observed 0+ states have been interpreted in terms of triple shape coexistence between spherical, oblate, and prolate deformed shapes. In the present work a new (02+) state at an energy of 1567 keV has been discovered in Ni70 by using β-delayed, γ-ray spectroscopy following the decay of Co70. The precipitous drop in the energy of the prolate-deformed 0+ level between Ni68 and Ni70 with the addition of two neutrons compares favorably with results of Monte Carlo shell-model calculations carried out in the large fpg9/2d5/2 model space, which predict a 02+ state at 1525 keV in Ni70. The result extends the shape-coexistence picture in the region to Ni70 and confirms the importance of the role of the tensor component of the monopole interaction in describing the structure of neutron-rich nuclei.

Shape coexistence near closed-shell nuclei, whereby states associated with deformed shapes appear at relatively low excitation energy alongside spherical ones, is indicative of the rapid change in structure that can occur with the addition or removal of a few protons or neutrons. Near 68Ni (Z=28, N=40), the identification of shape coexistence hinges on hitherto undetermined transition rates to and from low-energy 0+ states. In 68,70Ni, new lifetimes and branching ratios have been measured. These data enable quantitative descriptions of the 0+ states through the deduced transition rates and serve as sensitive probes for characterizing their nuclear wave functions. The results are compared to, and consistent with, large-scale shell-model calculations which predict shape coexistence. With the firm identification of this phenomenon near 68Ni, shape coexistence is now observed in all currently accessible regions of the nuclear chart with closed proton shells and mid-shell neutrons.