- He, Yu;
- Vishik, Inna M;
- Yi, Ming;
- Yang, Shuolong;
- Liu, Zhongkai;
- Lee, James J;
- Chen, Sudi;
- Rebec, Slavko N;
- Leuenberger, Dominik;
- Zong, Alfred;
- Jefferson, C Michael;
- Moore, Robert G;
- Kirchmann, Patrick S;
- Merriam, Andrew J;
- Shen, Zhi-Xun
We developed a table-top vacuum ultraviolet (VUV) laser with 113.778 nm wavelength (10.897 eV) and demonstrated its viability as a photon source for high resolution angle-resolved photoemission spectroscopy (ARPES). This sub-nanosecond pulsed VUV laser operates at a repetition rate of 10 MHz, provides a flux of 2 × 10(12) photons/s, and enables photoemission with energy and momentum resolutions better than 2 meV and 0.012 Å(-1), respectively. Space-charge induced energy shifts and spectral broadenings can be reduced below 2 meV. The setup reaches electron momenta up to 1.2 Å(-1), granting full access to the first Brillouin zone of most materials. Control over the linear polarization, repetition rate, and photon flux of the VUV source facilitates ARPES investigations of a broad range of quantum materials, bridging the application gap between contemporary low energy laser-based ARPES and synchrotron-based ARPES. We describe the principles and operational characteristics of this source and showcase its performance for rare earth metal tritellurides, high temperature cuprate superconductors, and iron-based superconductors.