Crows are omnivorous birds that feed on a wide range of natural and anthropogenic food sources. Consequently, they can cause considerable damage to crops and livestock feed; they also engage in garbage scavenging. The distribution of crow damage in environments with multiple fruits and vegetables is uneven, indicating potential food preferences. Although an understanding of food preferences is important for efforts to predict and mitigate the costs of damage caused by wild crows, few studies have investigated this phenomenon. We investigated the relationships between food preferences and foraging behaviors of wild-caught large-billed crows (Corvus macrorhynchos) through two experiments. Dry pet food for dogs (corn, meat powder, oils, and fats) and dried corn were used as favorable and less favorable experimental food types, respectively, based on previous field observations. In the first experiment, two feeding sites, each containing one of the food types, were placed at opposite ends of an outdoor U-shaped experimental cage (i.e., two-choice trial). In the second experiment, a single feeding site was established containing either pet food or dried corn (i.e., no-choice trial). Crows were placed in individual cages in both experiments. When both food types were available, large-billed crows foraged significantly more pet food than corn. There was no significant difference in consumption when either food type was presented alone, but total foraging duration was significantly longer for corn than for pet food. These results suggested that the amount of food consumed and foraging efficiency are good indicators of food preferences in large-billed crows under captive feeding conditions. Using this experimental approach, further studies are required to investigate the preferences of large-billed crows for a variety of food items, which will help to predict damage, improve trapping efficacy, and develop effective mitigation strategies.