- Xu, Cai-Zhi;
- Chan, Yang-Hao;
- Chen, Yige;
- Chen, Peng;
- Wang, Xiaoxiong;
- Dejoie, Catherine;
- Wong, Man-Hong;
- Hlevyack, Joseph Andrew;
- Ryu, Hyejin;
- Kee, Hae-Young;
- Tamura, Nobumichi;
- Chou, Mei-Yin;
- Hussain, Zahid;
- Mo, Sung-Kwan;
- Chiang, Tai-Chang
Three-dimensional (3D) topological Dirac semimetals (TDSs) are rare but important as a versatile platform for exploring exotic electronic properties and topological phase transitions. A quintessential feature of TDSs is 3D Dirac fermions associated with bulk electronic states near the Fermi level. Using angle-resolved photoemission spectroscopy, we have observed such bulk Dirac cones in epitaxially grown α-Sn films on InSb(111), the first such TDS system realized in an elemental form. First-principles calculations confirm that epitaxial strain is key to the formation of the TDS phase. A phase diagram is established that connects the 3D TDS phase through a singular point of a zero-gap semimetal phase to a topological insulator phase. The nature of the Dirac cone crosses over from 3D to 2D as the film thickness is reduced.