Background: Organic scintillators are widely used for neutron detection in both basic nuclear physics and applications. While the proton light yield of organic scintillators has been extensively studied, measurements of the light yield from neutron interactions with carbon nuclei are scarce. Purpose: Demonstrate a new approach for the simultaneous measurement of the proton and carbon light yield of organic scintillators. Provide new carbon light yield data for the EJ-309 liquid and EJ-204 plastic organic scintillators. Method: A 33-MeV H+2 beam from the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory was impinged upon a 3-mm-thick Be target to produce a high-flux, broad-spectrum neutron beam. The double time-of-flight technique was extended to simultaneously measure the proton and carbon light yields of the organic scintillators, wherein the light output associated with the recoil particle was determined using np and nC elastic scattering kinematics. Results: The proton and carbon light yield relations of the EJ-309 liquid and EJ-204 plastic organic scintillators were measured over a recoil energy range of approximately 0.3 to 1 MeV and 2 to 5 MeV, respectively, for EJ-309, and 0.2 to 0.5 MeV and 1 to 4 MeV, respectively, for EJ-204. Conclusions: These data provide new insight into the ionization quenching effect in organic scintillators and key input for simulation of the response of organic scintillators for both basic science and a broad range of applications.

Plastic, organic scintillators have been tailored in composition to achieve an ultrafast temporal response, thereby enabling the design and development of fast neutron detection systems with high timing resolution. Eljen Technology's plastic, organic scintillators- EJ-230, EJ-232, and EJ-232Q- are prospective candidates for use in emerging neutron imaging systems, where fast timing is paramount. To support the neutron response characterization of these materials, the relative proton light yields (PLYs) of EJ-230, EJ-232, and EJ-232Q were measured at the 88-Inch Cyclotron at the Lawrence Berkeley National Laboratory. Using a broad-spectrum neutron source and a double-Time-of-flight technique, the PLY relations were obtained over a proton recoil energy range of approximately 300 keV to 4 MeV. The EJ-230, EJ-232, and EJ-232Q scintillators exhibited similar PLY relations to each other and to other plastic scintillators with the same polymer base material. A comparison of the relative PLY of different sized cylindrical EJ-232 and EJ-232Q scintillators also revealed consistent results. This article provides key input data for the realistic computational modeling of neutron detection technologies employing these materials, thereby supporting new capabilities in near-field radionuclide detection for national security applications.

Compact neutron imagers using double-scatter kinematic reconstruction are being designed for localization and characterization of special nuclear material. These neutron imaging systems rely on scintillators with a rapid prompt temporal response as the detection medium. As n–p elastic scattering is the primary mechanism for light generation by fast neutron interactions in organic scintillators, proton light yield data are needed for accurate assessment of scintillator performance. The proton light yield of a series of commercial fast plastic organic scintillators – EJ-200, EJ-204, and EJ-208 – was measured via a double time-of-flight technique at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a tunable deuteron breakup neutron source, target scintillators housed in a dual photomultiplier tube configuration, and an array of pulse-shape-discriminating observation scintillators, the fast plastic scintillator light yield was measured over a broad and continuous energy range down to proton recoil energies of approximately 50 keV. This work provides key input to event reconstruction algorithms required for utilization of these materials in emerging neutron imaging modalities.

An organic glass scintillator developed by Sandia National Laboratories was characterized in terms of its light output and pulse shape discrimination (PSD) properties and compared to commercial liquid (EJ-309) and plastic (EJ-276) organic scintillators. The electron light output was determined through relative comparison of the 137Cs Compton edge location. The proton light yield was measured using a double time-of-flight technique at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. Using a tunable broad-spectrum neutron source and an array of pulse-shape-discriminating observation scintillators, a continuous measurement of the proton light yield was performed for EJ-309 (200 keV–3.2 MeV), EJ-276 (170 keV–4.9 MeV), and the organic glass (50 keV–20 MeV). Finally, the PSD properties of the organic glass, EJ-309, and EJ-276 were evaluated using an AmBe source and compared via a figure-of-merit metric. The organic glass exhibited a higher electron light output than both EJ-309 and EJ-276. Its proton light yield and PSD performance were comparable to EJ-309 and superior to that of EJ-276. With these performance characteristics, the organic glass scintillator is well poised to replace current state-of-the-art PSD-capable scintillators in a range of fast neutron detection applications.